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Ambient aerosol size distributions and number concentrations measured during the Pittsburgh Air Quality Study (PAQS)
Journal article   Open access   Peer reviewed

Ambient aerosol size distributions and number concentrations measured during the Pittsburgh Air Quality Study (PAQS)

Charles O Stanier, Andrey Y Khlystov and Spyros N Pandis
Atmospheric environment (1994), Vol.38(20), pp.3275-3284
2004
DOI: 10.1016/j.atmosenv.2004.03.020
url
https://doi.org/10.1016/j.atmosenv.2004.03.020View
Published (Version of record) Open Access

Abstract

Twelve months of aerosol size distributions from 3 to 560 nm, measured using scanning mobility particle sizers are presented with an emphasis on average number, surface, and volume distributions, and seasonal and diurnal variation. The measurements were made at the main sampling site of the Pittsburgh Air Quality Study from July 2001 to June 2002. These are supplemented with 5 months of size distribution data from 0.5 to 2.5 μm measured with a TSI aerosol particle sizer and 2 months of size distributions measured at an upwind rural sampling site. Measurements at the main site were made continuously under both low and ambient relative humidity. The average Pittsburgh number concentration (3–500 nm) is 22,000 cm −3 with an average mode size of 40 nm. Strong diurnal patterns in number concentrations are evident as a direct effect of the sources of particles (atmospheric nucleation, traffic, and other combustion sources). New particle formation from homogeneous nucleation is significant on 30–50% of study days and over a wide area (at least a hundred kilometers). Rural number concentrations are a factor of 2–3 lower (on average) than the urban values. Average measured distributions are different from model literature urban and rural size distributions.
 Urban air quality Number concentration Aerosol size distribution PAQS Pittsburgh Air Quality Study

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