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Chitosan conjugated with deoxycholic acid and gallic acid: A novel biopolymer-based additive antioxidant for polyethylene
Journal article   Open access   Peer reviewed

Chitosan conjugated with deoxycholic acid and gallic acid: A novel biopolymer-based additive antioxidant for polyethylene

Wanvimol Pasanphan, Garry R. Buettner and Suwabun Chirachanchai
Journal of applied polymer science, Vol.109(1), pp.38-46
07/05/2008
DOI: 10.1002/app.27953
url
https://doi.org/10.1002/app.27953View
Published (Version of record) Open Access

Abstract

Chitosan, as a novel bioadditive antioxidant for commodity polymer, is proposed. Chitosan is successfully conjugated with deoxycholic acid and gallic acid (chitosan-DC-GA) via a simple reaction using the 1-ethyl-3-(3'-dimethylaminopropyl) carbodiimide/N-hydroxysuccinimide conjugating agent at room temperature in a heterogeneous system. Chitosan-DC-GA shows a deoxycholic acid (DC) and gallic acid (GA) content of about 40% each. Chitosan-DC-GA exhibits DPPH radical scavenging ability with EC50 1 mg mL(-1) based on the EPR technique evaluation. A model case study of chitosan-DC-GA with low-density polyethylene (LDPE) confirms improvement in compatibility, as seen from the sheet clarity, as well as the good dispersion of chitosan-DC-GA in LDPE matrices, as observed by scanning electron microscope. (C) 2008 Wiley Periodicals, Inc.
Physical Sciences Polymer Science Science & Technology

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