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Effect of Sample Complexity on Quantification of Analytes in Aqueous Samples by Near-Infrared Spectroscopy
Journal article   Open access   Peer reviewed

Effect of Sample Complexity on Quantification of Analytes in Aqueous Samples by Near-Infrared Spectroscopy

Mark R Riley, Mark A Arnold and David W Murhammer
Applied spectroscopy, Vol.54(2), pp.255-261
02/2000
DOI: 10.1366/0003702001949186
url
https://doi.org/10.1366/0003702001949186View
Published (Version of record) Open Access

Abstract

This study was undertaken to quantitate the impact of increasing sample complexity on near-infrared spectroscopic (NIRS) measurements of small molecules in aqueous solutions with varying numbers of components. Samples with 2, 6, or 10 varying components were investigated. Within the 10-component samples, three analytes were quantified with errors below 6% and seven of the analytes were quantified with errors below 10%. An increase in the number of varying components can substantially increase the error associated with measurement. A comparison of measurement errors across sample sets, as gauged by the standard error of prediction (SEP), reveals that an increase in the number of varying components from 2 to 6 increases the SEP by approximately 50%. An increase from 2 to 10 varying components increases the SEP by approximately 340%. While there appear to be no substantial correlations between the presence of a specific analyte and the errors associated with quantification of another analyte, several analytes do display a small degree of sensitivity to varying concentrations of certain background components. The analysis also demonstrates that calibrations containing an overestimation of the numbers of varying components can substantially increase measurement errors and so calibrations must be constructed with an accurate understanding of the number of varying components that are likely to be encountered.
Quantification of analytes NIRS Aqueous solution Glucose Near-infrared spectroscopy

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