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Thiophene Derivative‐Loaded Nanoparticles Mediate Anticancer Activity Through the Inhibition of Kinases and Microtubule Assembly
Journal article   Peer reviewed

Thiophene Derivative‐Loaded Nanoparticles Mediate Anticancer Activity Through the Inhibition of Kinases and Microtubule Assembly

Somaya A Abdel‐Rahman, Emad I Wafa, Kareem Ebeid, Sean M Geary, Youssef W Naguib, Ashraf K El‐Damasy and Aliasger K Salem
Advanced therapeutics, Vol.4(7), pp.2100058-n/a
07/2021
DOI: 10.1002/adtp.202100058
PMCID: PMC8372755
PMID: 34423112
url
https://www.ncbi.nlm.nih.gov/pmc/articles/8372755View
Open Access

Abstract

Different tetrahydrobenzo[b]thiophene derivatives are explored as new tubulin polymerization destabilizers to arrest tumor cell mitosis. A series of compounds incorporating the tetrahydrobenzo[b]thiophene scaffold are synthesized, and their biological activities are investigated. The cytotoxicity of each of the synthesized compounds is assessed against a range of cell lines. Specifically, the benzyl urea tetrahydrobenzo[b]thiophene derivative, 1-benzyl-3-(3-cyano-4,5,6,7-tetrahydrobenzo[b]thiophen-2-yl)urea (BU17), is identified as the most potent compound with broad-spectrum antitumor activity against several cancer cell lines. The potential mechanism(s) of action are investigated where dose-dependent G2/M accumulation and A549 cell cycle arrest are detected. Additionally, A549 cells treated with BU17 express enhanced levels of caspase 3 and 9, indicating the induction of apoptosis. Furthermore, it is found that BU17 inhibits WEE1 kinase and targets tubulin by blocking its polymerization. BU17 is also formulated into PLGA nanoparticles, and it is demonstrated that BU17-loaded nanoparticles can significantly enhance antitumor activity compared to the soluble counterpart.

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