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Single Color Center Spin Coherence revealed in Optically Detected Magnetic Resonance of an Ensemble of Silicon Vacancies in SiC
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Single Color Center Spin Coherence revealed in Optically Detected Magnetic Resonance of an Ensemble of Silicon Vacancies in SiC

David A Fehr, Hannes Kraus, Corey J Cochrane and Michael E Flatté
ArXiv.org
Cornell University
11/30/2025
DOI: 10.48550/arxiv.2512.01144
url
https://doi.org/10.48550/arxiv.2512.01144View
Preprint (Author's original)This preprint has not been evaluated by subject experts through peer review. Preprints may undergo extensive changes and/or become peer-reviewed journal articles. Open Access

Abstract

We present a quantitative theory for simulating optically detected magnetic resonance (ODMR) measurements of optically-active spin centers using steady-state Lindblad equations. We apply the theory to an experimental ODMR spectrum associated with the negatively-charged silicon vacancy V2 center in 6H-SiC, showing that spin Hamiltonian parameters, optical transition rates, and even coherence times may be extracted, with values consistent with recent literature. Notably the T2 spin coherence time is measurable, not just the T ∗ 2 dephasing time. Furthermore, we simulate the ODMR spectra of a V2 center in isotopically-purified 6H-SiC, and predict an order-of-magnitude narrowing of some, but not all spectral lines compared with natural abundance samples.
Physics - Mesoscale and Nanoscale Physics

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